Unconventional Magnetism via Optical Pumping of Interacting Spin Systems

Unconventional magnetism via optical pumping of interacting spin systems.

We consider strongly interacting systems of effective spins, subject to dissipative spin-flip processes associated with optical pumping. We predict the existence of novel magnetic phases in the steady state of this system, which emerge due to the competition between coherent and dissipative processes. Specifically, for strongly anisotropic spin-spin interactions, we find ferromagnetic, antiferr...

Fundamentals of Spin-Exchange Optical Pumping

The standard model of Spin-Exchange Optical Pumping of He has come under close scrutiny as researchers try to maximize the quantity and polarization of He. This paper will review four important effects that have come to light: 1) pumping with frequency narrowed diode lasers significantly improves the polarization and production rate as compared to off-theshelf broadband sources 2) Rb-K mixtures...

Hybrid spin-exchange optical pumping of 3He.

We demonstrate spin-exchange optical pumping of 3He using a "hybrid" K-Rb vapor mixture. The Rb atoms absorb light from a standard laser at 795 nm, then collisionally polarize the potassium atoms. Spin-exchange collisions of K and 3He atoms then transfer the angular momentum to the 3He with much greater efficiency than Rb-3He. For a K-rich vapor, the efficiency of the hybrid spin-exchange colli...

Temperature-Ramped 129Xe Spin-Exchange Optical Pumping

We describe temperature-ramped spin-exchange optical pumping (TR-SEOP) in an automated high-throughput batch-mode (129)Xe hyperpolarizer utilizing three key temperature regimes: (i) "hot"-where the (129)Xe hyperpolarization rate is maximal, (ii) "warm"-where the (129)Xe hyperpolarization approaches unity, and (iii) "cool"-where hyperpolarized (129)Xe gas is transferred into a Tedlar bag with lo...

Spin-Exchange optical pumping in a van